I believe the tail rotor or the tail boom visually failed first. Although this could be due to main transmission mount failure or similar and the transmission twisting around.
In the video at 5:37 in Juan's presentation, the helicopter seems to sharply yaw right, followed by in flight breakup. The tail sure seems to depart first, then the main rotor system. At 7:12 the main rotor is seen directly above the fuselage.
In more compete videos, the tail boom seems to be far behind the main rotor.
In any case, these transmissions are well attached, and known to be structurally able to handle about 6G's of force without damage. The heli is certified to (I believe) 3.5G, and the structural design limit is always 150% or more than the certification limit or about 5.25G. I am not at all sure the blades can, even briefly, generate more lift than that without stalling.
For that transmission and tailboom to come off so rapidly it is likely forms of weaknesses existed. Corrosion and fatigue always come to mind on a 20+ year old tour helicopter.